Recent status of the cryogenic sample environment at the MLF, J-PARC

Ishikado, Motoyuki*; Takahashi, Ryuta*; Yamauchi, Yasuhiro*; Nakamura, Masatoshi*; Ishimaru, Sora*; Yamauchi, Sara*; Kawamura, Seiko; Kira, Hiroshi*; Sakaguchi, Yoshifumi*; Watanabe, Masao; et al.

JPS Conference Proceedings (Internet), 41, p.011010_1 - 011010_7, 2024/05

https://doi.org/10.7566/JPSCP.41.011010

A Science-based mixed oxide property model for developing advanced oxide nuclear fuels

Kato, Masato; Oki, Takumi; Watanabe, Masashi; Hirooka, Shun; Vauchy, R.; Ozawa, Takayuki; Uwaba, Tomoyuki; Ikusawa, Yoshihisa; Nakamura, Hiroki; Machida, Masahiko

Journal of the American Ceramic Society, 107(5), p.2998 - 3011, 2024/05

https://doi.org/10.1111/jace.19609

Replacement of incinerator adopted to Plutonium Waste Treatment Facility

Yamashita, Kiyoto; Maki, Shota; Yokosuka, Kazuhiro; Fukui, Masahiro; Iemura, Keisuke

JAEA-Technology 2023-023, 97 Pages, 2024/03

JAEA-Technology-2023-023.pdf:8.21MB

The incinerator adopted to incineration room, Plutonium Waste Treatment Facility had been demonstrated since 2002 for developing technologies to reduce the volume of fire-resistant wastes such as vinyl chloride (represented by Polyvinyl chloride bags) and rubber gloves for Radio Isotope among radioactive solid wastes generated by the production of mixed oxide fuels. The incinerator, cooling tower, and processing pipes were replaced with a suspension period from 2018 to 2022, which fireproof materials on the inner wall of the incinerator was cracked and grown caused by hydrogen chloride generated when disposing of fire-resistant wastes. This facility consists of the waste feed process, the incineration process, the waste gas treatment process, and the ash removal process. We replaced the cooling tower in the waste gas treatment process from March 2020 to March 2021, and the incinerator in the incineration process from January 2021 to February 2022. In addition, samples were collected from the incinerator and the cooling tower during the removing and dismantling of the replaced devices, observed by Scanning Electron Microscope and X-ray microanalyzer, and analyzed by X-ray diffraction to investigate the corrosion and deterioration of them. This report describes the method of setting up the green house, the procedure for replacing them, and the results from analysis in corrosion and deterioration of the cooling tower and incinerator.

Stress measurement of stainless steel piping welds by complementary use of high-energy synchrotron X-rays and neutrons

Miura, Yasufumi*; Suzuki, Kenji*; Morooka, Satoshi; Shobu, Takahisa

Quantum Beam Science (Internet), 8(1), p.1_1 - 1_14, 2024/03

https://doi.org/10.3390/qubs8010001

Anisotropic electrical conductivity changes in FeTiO structure transition under high pressure

Yamanaka, Takamitsu*; Nakamoto, Yuki*; Sakata, Masafumi*; Shimizu, Katsuya*; Hattori, Takanori

Physics and Chemistry of Minerals, 51(1), p.4_1 - 4_10, 2024/02

https://doi.org/10.1007/s00269-023-01261-6

Neutron and synchrotron X-ray diffraction and electric conductivity measurements of FeTiO ilmenite were performed under pressures. Ilmenite structure is retained up to 28 GPa. Structure analysis revealed that FeO and TiO are compressible and less compressible below 8 GPa, respectively. The resistivity is lowest along the Fe-Ti direction that has shortest interatomic distance among all the metal ion pairs. The resistivity in the direction normal to c-axis monotonically decreases with pressure, whereas that along c-axis shows hallow-shape with pressure. Maximum entropy analysis shows that electron configuration of Fe (3) is more strongly changed than Ti (3) under compression. The anisotropic electrical conductivity and non-uniform structure change of Fe-Ti interatomic distance can be explained by the possible spin transition from high-spin state to intermediate-spin state of Fe cation.

Probing deformation behavior of a refractory high-entropy alloy using neutron diffraction

Zhou, Y.*; Song, W.*; Zhang, F.*; Wu, Y.*; Lei, Z.*; Jiao, M.*; Zhang, X.*; Dong, J.*; Zhang, Y.*; Yang, M.*; et al.

Journal of Alloys and Compounds, 971, p.172635_1 - 172635_7, 2024/01

https://doi.org/10.1016/j.jallcom.2023.172635

Neutron flux estimation and neutronics characteristics calculation in post-JMTR conceptual study

Oizumi, Akito; Akie, Hiroshi

JAEA-Technology 2023-017, 93 Pages, 2023/12

JAEA-Technology-2023-017.pdf:8.45MB

After the decision of decommissioning JMTR (Japan Materials Testing Reactor), Japan Atomic Energy Agency investigated the possibility to construct a new irradiation test reactor to succeed JMTR (post-JMTR), and the final report of the investigated result was submitted to the Ministry of Education, Culture, Sports, Science and Technology on March 30th 2021. This investigation was carried out in 4 steps of (1) selection of reactor type, (2) reactor core plans studies, (3) neutronic studies, (4) thermal studies, and was finally (5) considered and evaluated. This JAEA-Technology report summarizes the process and the results of (3) neutronic studies. Neutron fluxes were calculated at irradiation sample positions in the investigated cores, the standard core and the compact core, and the calculated fluxes satisfied the required irradiation capability. It was also evaluated the two investigated cores' continuous reactor operation time in days in one refueling cycle, and the results guaranteed an operation days equality with that of existing JMTR. In addition, neutronic characteristics of the cores were estimated, such as power distribution in the core, control rod reactivity worth, reactivity coefficients, distribution of fuel burnup rate of each fuel element, and kinetics parameters. The evaluated neutronic characteristics were used in the post-JMTR final investigation report to confirm the neutronic feasibility by comparing with the neutronic limiting values of existing JMTR, and to estimate the cooling capability to make the core thermally feasible.

Summaries of research and development activities by using supercomputer system of JAEA in FY2022 (April 1, 2022 - March 31, 2023)

HPC Technology Promotion Office

JAEA-Review 2023-018, 159 Pages, 2023/12

JAEA-Review-2023-018.pdf:13.62MB

Japan Atomic Energy Agency (JAEA) conducts research and development (R&D) in various fields related to nuclear power as a comprehensive institution of nuclear energy R&Ds, and utilizes computational science and technology in many activities. Over the past 10 years or so, the publication of papers utilizing computational science and technology at JAEA has accounted for about 20 percent of the total publications each fiscal year. The supercomputer system of JAEA has become an important infrastructure to support computational science and technology. In FY2022, the system was used for R&D of light water reactors, high-temperature gas reactors, and fast reactors to contribute to carbon neutrality as a priority issue, as well as for JAEA's major projects such as Various R&D related to nuclear science and technology, R&D related to the response to the accident at TEPCO's Fukushima Daiichi Nuclear Power Station, Development of technology for treatment and disposal of high-level radioactive waste, Support of nuclear safety regulation and nuclear disaster prevention, and safety research for this purpose. This report presents a great number of R&D results accomplished by using the system in FY2022, as well as user support, operational records and overviews of the system, and so on.

Estimation of continuous distribution of iterated fission probability using an artificial neural network with Monte Carlo-based training data

Tuya, D.; Nagaya, Yasunobu

Journal of Nuclear Engineering (Internet), 4(4), p.691 - 710, 2023/11

https://doi.org/10.3390/jne4040043

The Monte Carlo method is used to accurately estimate various quantities such as k-eigenvalue and integral neutron flux. However, when a distribution of a quantity is desired, the Monte Carlo method does not typically provide continuous distribution. Recently, the functional expansion tally and kernel density estimation methods have been developed to provide continuous distribution. In this paper, we propose a method to estimate a continuous distribution of a quantity using artificial neural network (ANN) model with Monte Carlo-based training data. As a proof of concept, a continuous distribution of iterated fission probability (IFP) is estimated by ANN models in two systems. The IFP distributions by the ANN models were compared with the Monte Carlo-based data and the adjoint angular neutron fluxes by the PARTISN code. The comparisons showed varying degrees of agreement or discrepancy; however, it was observed that the ANN models learned the general trend of the IFP distributions.

Measurements of capture cross-section of Nb by activation method and half-life of Nb by mass analysis

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi

Journal of Nuclear Science and Technology, 60(11), p.1361 - 1371, 2023/11

https://doi.org/10.1080/00223131.2023.2198526

The thermal-neutron capture cross section () and resonance integral (I) for Nb among nuclides for decommissioning were measured by an activation method and the half-life of Nb by mass analysis. Niobium-93 samples were irradiated with a hydraulic conveyer installed in the research reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Gold-aluminum, cobalt-aluminum alloy wires were used to monitor thermal-neutron fluxes and epi-thermal Westcott's indexes at an irradiation position. A 25-m-thick gadolinium foil was used to sort out reactions ascribe to thermal-and epi-thermal neutrons. Its thickness provided a cut-off energy of 0.133 eV. In order to attenuate radioactivity of Ta due to impurities, the Nb samples were cooled for nearly 2 years. The induced radio activity in the monitors and Nb samples were measured by -ray spectroscopy. In analysis based on Westcott's convention, the and I values were derived as 1.110.04 barn and 10.50.6 barn, respectively. After the -ray measurements, mass analysis was applied to the Nb sample to obtain the reaction rate. By combining data obtained by both -ray spectroscopy and mass analysis, the half-life of Nb was derived as (2.000.15)10 years.